Across
- 1. Online cult in Falcon and the Winter Soldier
- 6. Hulk villain who wanted to take down the president in Captain America 4
- 8. Scientist variant of Doc Ock in Spider-Man: Into the Spider-Verse
- 10. Comic-booky villain of Spider-Man 4
- 12. Comic-booky villain of the first Ant-Man
- 13. Variant of He Who Remains in season 2 of Loki
- 14. Comic-booky villain of Black Widow
- 15. Squidward [Iron Man nickname "Squidward" refers to which leader of the Black Order in Infinity War]
- 16. Mutant leader of the Hand in Elektra
- 17. Wolverine's Brother in Origins
- 18. God-Butcher in Thor 4
- 21. Villain of first Venom movie
- 23. Villain of She-Hulk and wife of Absorbing Man
- 24. Mayor and overall Daredevil: Born Again Season 2
- 28. Twin of Professor X and villain of Deadpool's third movie
- 30. Judgy villain in Moon Knight
- 31. Twist villain of WandaVision
- 34. Peter's friend and the murderer of Gwen Stacy in Amazing Spider-Man sequel
- 36. Title villain of Venom sequel
- 38. First villain of the Guardians of the Galaxy
- 43. Thor's sister in his third movie
- 44. Final villain of Jessica Jones's comic name
- 45. Villain of the week of Into the Spider-Verse sequel
- 46. The tech corporation formed in Iron Man 3
- 50. First villain of the Amazing Spider-Man
- 51. Final villain of the Avengers in the Infinity Saga
- 55. Computer that appeared as their comic book form in Captain America: The Winter Soldier
- 57. This villain got a spinoff show where they fight the Kingpin of crime
- 59. Twist villain in Doctor Strange sequel
- 60. AI villain of Agents of S.H.I.E.L.D. Season 4
- 61. Kid in Deadpool sequel
- 62. Agent Carter Recurring villain
- 65. The human "villain" of the Inhumans who wanted the humans to be treated slightly better and not be slaves
- 70. Villain of first ever Spider-Man movie
- 71. Doctor in the New Mutants
- 72. FBI agent who works for Fisk in final season of original Daredevil show
- 74. Watery villain of the Black Panther sequel
- 76. Name of the suit of the villain in Iron Man
- 80. Villain that brought together the Avengers
- 81. Computer in Captain Marvel
- 83. Teased villain of final Venom movie
- 87. Comic booky villain of final Blade movie
- 89. Mastermind ninja villain of first season of Iron Fist
- 90. Villain who appeared shortly in Daredevil: Born Again Season 1 whose love of art was so passionate, it's a crime
- 91. Jessica Jones's mom in Season 2 of her show
- 96. Man Drax and Mantis were tasked to chase after in Holiday Special and also killed Magneto's parents
- 97. T'Challa's cousin in his first movie
- 98. The only villain who actually didn't know Peter Parker is Spider-Man in Spider-Man: No Way Home
- 99. Comic-booky character who was the villain of the Agents of S.H.I.E.L.D. pilot
- 101. Scientist who created Wolverine and returned in X2
- 102. Final villain of Season 1 of Loki
- 103. Corporation that ruins Cloak and Dagger's life in first season
- 104. Only surviving family member of the Gnucchi family who swore vengeance on Castle in One Last Kill
- 105. The armor that attacks Thor in his origin movie
- 106. Fireball villain of Dr. Strange
- 107. First villain of Blade
- 108. Comic-booky female villain of Iron Fist Season 2
- 109. Assassin in Ben Affleck Daredevil movie
- 110. Fantastic Four: First Steps Villain
Down
- 2. Villain of final Guardians of the Galaxy movie
- 3. Villain of Blade sequel
- 4. Villain of original 2000's Fantastic Four
- 5. Twist villain of the finale of Agents of S.H.I.E.L.D. Season 5
- 7. Super-Skrull in Secret Invasion
- 9. Title villain of Avengers sequel
- 11. Villain in Europe in Spider-Man: Far From Home
- 15. Peter Quill's father
- 19. Comic book name of the villain of Punisher Season 1
- 20. Monster villain of Kraven the Hunter
- 22. Shang-Chi's father in his first movie
- 25. Villain of first MCU Spider-Man movie, he's not Batman, he's not Birdman, he's the ____
- 26. Overall villain of the first X-Men
- 27. Successor of Ronan in the Marvels
- 29. Original villain of the Multiverse Saga but only was in third Ant-Man movie
- 32. Villain who gave Wade Wilson his powers
- 33. This alien who was played by Clark Gregg was referred to as the ____
- 35. Reoccuring villain Luke Cage Season 2
- 37. Company created by Tony Stark that chased after the Wonder Man
- 39. Villain of the pilot of Luke Cage
- 40. Overall villain of Iron Heart
- 41. Teased villain in Hawkeye
- 42. Name of crime boss in the first episode of Daredevil
- 47. Title villain of Fantastic Four sequel
- 48. Comic-booky villain in the pilot of Agents of S.H.I.E.L.D. Season 2
- 49. Vampire villain of Morbious
- 52. X-Men: First Class Villain
- 53. Evil clone detective in the final season of Cloak and Dagger
- 54. Villain of Eyes of Wakanda pilot
- 56. Murderer of Ben Parker in Spider-Man 3
- 58. Creator of H.Y.D.R.A. in Agents of S.H.I.E.L.D. Season 3
- 63. Captain America: First Avenger villain
- 64. Ex of Agatha and villain of her show
- 66. Cybernetic Wolverine in the movie Logan
- 67. General in Incredible Hulk
- 68. Thor sequel villain who wanted "Darkness", I guess
- 69. Giant mech at the end of The Wolverine
- 70. Comic-booky villain of Ant-Man and the Wasp
- 72. Villain of third Captain America movie
- 73. Twist villain of Eternals
- 75. Sentry's second side that destroyed the city in the Thunderbolts
- 77. Finish the quote from X3: "I'm the _____, B****
- 78. Daredevil's girlfriend and recurring villain of season 2 of his show
- 79. Relative of Elsa and villain of Werewolf by Night
- 82. The kid the Agents of S.H.I.E.L.D. were sent back in time to protect in the final season of their show
- 83. Telepathic in the first season of Jessica Jones
- 84. Guy Who Created Robots in Days of Future Past
- 85. Billionaire in Iron Man 2
- 86. Group of magic evil SECRET people in Ms. Marvel
- 88. Punisher Season 2 religious villain
- 92. Ninja cult who the Defenders fight
- 93. Title villain of 90's X-Men Movie
- 94. Villain of the best Spider-Man sequel
- 95. ADRd villain of Madame Web
- 100. Title villain of 80's X-Men Movie